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• W2908888041 abstract "A new diradical having two 4,8,10-trioxotriangulene (TOT) neutral radical units linked through an m-phenylene moiety was synthesized and characterized by ESR measurements. An electrochemical study showed that the diradical undergoes two one-electron reductions to generate corresponding dianion species, suggesting the electronic interaction between two TOT units through the π-conjugated spacer. A strong intramolecular interaction between the two TOT units gives rise to the spin-projected small hyperfine couplings in comparison with those of the monomer. Furthermore, the temperature dependent ESR measurement revealed that the dimer behaves as an S=1 species in the ground state with a ferromagnetic interaction of 2 J/kB =+7±3 K." @default.
• W2908888041 created "2019-01-25" @default.
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• W2908888041 date "2019-01-28" @default.
• W2908888041 modified "2023-10-01" @default.
• W2908888041 title "Intramolecular Magnetic Interaction of Spin‐Delocalized Neutral Radicals through <i>m</i> ‐Phenylene Spacers" @default.
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• W2908888041 doi "https://doi.org/10.1002/cplu.201800662" @default.
• W2908888041 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31944024" @default.
• W2908888041 hasPublicationYear "2019" @default.
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