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- W2909181386 abstract "Abstract Palladium-catalyzed cross-coupling reactions are one of the most powerful and versatile methods to synthesize a wide range of complex functionalized molecules. However, the development of solid-state cross-coupling reactions remains extremely limited. Here, we report a rational strategy that provides a general entry to palladium-catalyzed Buchwald-Hartwig cross-coupling reactions in the solid state. The key finding of this study is that olefin additives can act as efficient molecular dispersants for the palladium-based catalyst in solid-state media to facilitate the challenging solid-state cross-coupling. Beyond the immediate utility of this protocol, our strategy could inspire the development of industrially attractive solvent-free palladium-catalyzed cross-coupling processes for other valuable synthetic targets." @default.
- W2909181386 created "2019-01-25" @default.
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- W2909181386 date "2019-01-10" @default.
- W2909181386 modified "2023-10-17" @default.
- W2909181386 title "Olefin-accelerated solid-state C–N cross-coupling reactions using mechanochemistry" @default.
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- W2909181386 doi "https://doi.org/10.1038/s41467-018-08017-9" @default.
- W2909181386 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6328594" @default.
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- W2909181386 hasPublicationYear "2019" @default.
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