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- W2909212595 abstract "Streams of waste mixed acids from conventional wet etching processes contain high levels of H3PO4, which warrant recycling. This investigation is the first to use metal organic framework UiO-66 and UiO-66-NH2 to adsorb phosphoric acid from waste mixed acids from the world's largest semiconductor foundry, a synthetic HNO3H3PO4HAc mixture, and 85% phosphoric acid. Both UiO-66 and UiO-66-NH2 have high capacities to adsorb H3PO4 in extremely acidic solutions. The Langmuir adsorption capacities (qmax’s) of UiO-66 for waste mixed acids and a synthetic HNO3H3PO4HAc mixture on UiO-66 at 25 °C are 3360 and 8,510 mg-H3PO4/g, respectively, and that of 85% phosphoric acid on UiO-66 is 4,790 mg-H3PO4/g. The qmax of UiO-66-NH2 for phosphoric acid from 25% to 75% waste mixed acids is 4550 mg-H3PO4/g, which exceeds that of UiO-66. The corresponding P:Zr ratio for adsorbed MOF is in the range 6.2‒13.5, suggesting that the tested MOF crystals are super-adsorbents of phosphoric acid under extremely acidic conditions." @default.
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- W2909212595 date "2019-03-01" @default.
- W2909212595 modified "2023-09-23" @default.
- W2909212595 title "Effective adsorption of phosphoric acid by UiO-66 and UiO-66-NH2 from extremely acidic mixed waste acids: Proof of concept" @default.
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- W2909212595 doi "https://doi.org/10.1016/j.jtice.2018.12.018" @default.
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