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• W2909342015 abstract "Abstract The thermal gas‐phase reactions of [Al 2 VO 5 ] + and [AlV 2 O 6 ] + with methane have been explored by using Fourier transform ion cyclotron resonance (FT‐ICR) mass spectrometry complemented by high‐level quantum chemical calculations. Both cluster ions chemisorbed methane as the major reaction channels at room temperature. [Al 2 VO 5 ] + could break only one C−H bond to liberate CH 3 , whereas [AlV 2 O 6 ] + exhibited higher oxidizing ability such that it brings about the selective generation of formaldehyde. Mechanistic aspects are revealed and the crucial roles of the metal centers are discussed." @default.
• W2909342015 created "2019-01-25" @default.
• W2909342015 creator A5003216863 @default.
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• W2909342015 date "2019-02-07" @default.
• W2909342015 modified "2023-10-01" @default.
• W2909342015 title "Tuning the Reactivities of the Heteronuclear [Al_<i>n</i> V_3−<i>n</i> O_7−<i>n</i> ]⁺ (<i>n=</i> 1, 2) Cluster Oxides towards Methane by Varying the Composition of the Metal Centers" @default.
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• W2909342015 doi "https://doi.org/10.1002/chem.201805908" @default.
• W2909342015 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30659675" @default.
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