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- W2910250933 abstract "Incorporation of 226Ra within gypsum (CaSO4·2H2O(s)) and celestite (SrSO4(s)) was assessed through dedicated batch experiments monitored over hundreds of days. Dissolution/recrystallization and coprecipitation experiments were carried out to investigate a range of chemical conditions, close to or far from equilibrium conditions. These data were used to establish the ability of gypsum and celestite to incorporate 226Ra. Celestite shows a high 226Ra incorporation, with a partition coefficient around 105. On the contrary, 226Ra is not significantly incorporated into pure gypsum. A very low value of (8.8 ± 1.5) × 10–4 has been estimated, which is much lower than the values reported in the literature. This may explain why 226Ra incorporation in gypsum is enhanced when Sr impurities are present (above 0.1 molar %). Under such conditions, the radium distribution coefficient is around 0.15 ± 0.09. This behavior can be explained by an ion-exchange mechanism between 226Ra and Sr, consistently with the existence of ..." @default.
- W2910250933 created "2019-01-25" @default.
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- W2910250933 date "2019-01-16" @default.
- W2910250933 modified "2023-10-18" @default.
- W2910250933 title "Role of Trace Elements in the 226-Radium Incorporation in Sulfate Minerals (Gypsum and Celestite)" @default.
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- W2910250933 doi "https://doi.org/10.1021/acsearthspacechem.8b00150" @default.
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