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• W2910558775 endingPage "5001" @default.
• W2910558775 startingPage "4993" @default.
• W2910558775 abstract "Phosphoryl ligands of the general formula O═PR3 (R = Me, OMe, Et, nBu, Ph, iPr, NMe2) were coordinated to [Nd(TriNOx)] (TriNOx3– = ([(2-tBuNO)C6H4CH2]3N)3–), and the resulting complexes were characterized. Solution equilibrium constants for each complex were determined, demonstrating a large range for phosphoryl ligands’ Lewis basicity. Thermogravimetric analyses provided evidence for the qualitative thermodynamic preference of phosphoryl ligands for [Nd(TriNOx)] over the dysprosium analogue. These findings were exploited for the separation of binary mixtures of neodymium/dysprosium and lanthanum/neodymium. Implementation of phosphoryl ligands in the TriNOx separation system expands its scope and demonstrates a fundamentally different mode for separating rare-earth cations based on adducts with neutral donors." @default.
• W2910558775 created "2019-01-25" @default.
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• W2910558775 date "2019-01-18" @default.
• W2910558775 modified "2023-10-14" @default.
• W2910558775 title "Phosphoryl-Ligand Adducts of Rare Earth-TriNOx Complexes: Systematic Studies and Implications for Separations Chemistry" @default.
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• W2910558775 doi "https://doi.org/10.1021/acssuschemeng.8b05638" @default.
• W2910558775 hasPublicationYear "2019" @default.
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