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• W2910646744 abstract "We performed a series of plate impact experiments on NH3 gas initially at room temperature and at a pressure of ∼100 psi. Shocked states were determined by optical velocimetry and the temperatures by optical pyrometry, yielding compression ratios of ∼5–10 and second shock temperatures in excess of 7500 K. A first-principles statistical mechanical (thermochemical) approach that included chemical dissociation yielded reasonable agreement with experimental results on the principal Hugoniot, even with interparticle interactions neglected. Theoretical analysis of reshocked states, which predicts a significant degree of chemical dissociation, showed reasonable agreement with experimental data for higher temperature shots; however, reshock calculations required the use of interaction potentials. We rationalize the very different shock temperatures obtained, relative to previous results for argon, in terms of atomic versus molecular heat capacities." @default.
• W2910646744 created "2019-01-25" @default.
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• W2910646744 date "2019-01-08" @default.
• W2910646744 modified "2023-10-16" @default.
• W2910646744 title "Shockwave compression and dissociation of ammonia gas" @default.
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• W2910646744 doi "https://doi.org/10.1063/1.5063012" @default.
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