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- W2910852017 abstract "A series of solid acid WO 3 /TiO 2 ‐supported lithium‐manganese oxide (Li‐Mn/WO 3 /TiO 2 ) catalysts for the oxidative coupling of methane (OCM) were prepared by the impregnation method. The XRD and XPS analyses showed that increasing the calcination temperature could promote the generation of Mn 2+ and Mn 3+ species and the anatase‐to‐rutile phase transformation of TiO 2 , which are beneficial to the OCM reaction. It was revealed by CO 2 ‐TPD, O 2 ‐TPD, H 2 ‐TPR, XPS, and CH 4 ‐TPSR that Li‐Mn/WO 3 /TiO 2 with higher calcination temperature possessed much stronger surface basicity, lower lattice oxygen mobility, and more abundant lattice oxygen, which are favorable for the selectivity to C 2 hydrocarbons. The catalytic, structural, and spectroscopic results showed that the catalytic performance, structure, and properties of catalysts were little influenced by the calcination temperature of the WO 3 /TiO 2 support. The optimized calcination temperature of the support and the catalyst is 800 °C, on which the highest C 2 yield of 16.3 % was achieved at a reaction temperature of 750 °C." @default.
- W2910852017 created "2019-01-25" @default.
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- W2910852017 date "2019-02-12" @default.
- W2910852017 modified "2023-09-25" @default.
- W2910852017 title "Effect of Calcination Temperature on the Characteristics and Performance of Solid Acid WO <sub>3</sub> /TiO <sub>2</sub> ‐Supported Lithium‐Manganese Catalysts for the Oxidative Coupling of Methane" @default.
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- W2910852017 doi "https://doi.org/10.1002/ejic.201801427" @default.
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