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• W2911592169 endingPage "9461" @default.
• W2911592169 startingPage "9448" @default.
• W2911592169 abstract "We demonstrated a novel mixed-matrix composite membrane (MMCM) based on acrylated polyurethane (APU) and UiO-66 nanoparticles to separate CO2/N2 mixture. UiO-66 and functionalized UiO-66 including NH2-UiO-66 and glycidyl methacrylate (GMA)-UiO-66 were loaded into APU/2-hydroxyethyl methacrylate (APUH) matrix at variable concentrations between 3 and 30 wt %. APUH/GMA-UiO-66 MMCMs exhibited strong adhesion with a support layer of polyester/polysulfone, which was not deteriorated after immersion in water for a long time (20 days). Incorporation of UiO-66 and its functionalized forms increased simultaneously permeability and CO2/N2 selectivity, which were indeed superior in comparison with those of MMCMs reported previously. GMA-UiO-66-filled MMCM displayed a CO2 permeance of 14.5 Barrer and a CO2/N2 selectivity of 53 at a critical concentration (25 wt %). This attractive separation performance of APUH/UiO-66 offered an exciting platform for the development of composite membranes for sustainable CO2 separations." @default.
• W2911592169 created "2019-02-21" @default.
• W2911592169 creator A5034539950 @default.
• W2911592169 creator A5047336732 @default.
• W2911592169 date "2019-02-06" @default.
• W2911592169 modified "2023-09-26" @default.
• W2911592169 title "Mixed-Matrix Composite Membranes Based on UiO-66-Derived MOFs for CO₂ Separation" @default.
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• W2911592169 doi "https://doi.org/10.1021/acsami.8b20869" @default.
• W2911592169 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30724557" @default.
• W2911592169 hasPublicationYear "2019" @default.
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