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- W2912013163 abstract "Highly selective detection of trace metal ions has become one of the most urgent issues in public security and living systems. Developing a highly efficient fluorescent sensor for manganese(ii) (Mn2+) ions is a huge challenge. Herein, by utilizing the solvent regulation approach, a pair of terbium metal-organic frameworks (UPC-36, [Tb2(btdc)3(DMF)(H2O)4]·DMF and UPC-37, [Tb2(btdc)3(H2O)6]) based on a π-electron-rich ligand (H2btdc = 2,2'-bithiophene-5,5'-dicarboxylic acid) has been chosen as highly efficient sensors for the selective detection of Mn2+ ions. Interestingly, the fluorescence of UPC-36 can be quenched by Mn2+, Cu2+, Al3+, Cr3+ and Fe3+ ions, while UPC-37 can only be quenched by Mn2+ ions. For detecting Mn2+ ions, the limit of detection (LOD) values are calculated to be 0.813 mM and 0.715 mM for UPC-36 and UPC-37 respectively. According to the ICP results, UPC-37 has stronger interactions with Mn2+ ions because of the more regular arrangement of ligands existing in UPC-37, so it exhibits a high sensitivity and selectivity (Ksv = 5.25 × 105 M-1)." @default.
- W2912013163 created "2019-02-21" @default.
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- W2912013163 date "2019-01-01" @default.
- W2912013163 modified "2023-10-15" @default.
- W2912013163 title "Solvent-induced terbium metal–organic frameworks for highly selective detection of manganese(<scp>ii</scp>) ions" @default.
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- W2912013163 doi "https://doi.org/10.1039/c9dt00006b" @default.
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