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• W2912018790 abstract "Ion transport through nanopores is a process of fundamental significance in nature and in engineering practice. Over the past decade, it has been found that the ion conductivity in nanopores could be drastically enhanced, and different mechanisms have been proposed to explain this observation. To date, most reported studies have been carried out with relatively dilute electrolytes, while ion transport in nanopores under high electrolyte concentrations (>1 M) has been rarely explored. Through systematic experimental and atomistic simulation studies with NaCl solutions, here we show that at high electrolyte concentrations, ion mobility in small nanopores could be significantly reduced from the corresponding bulk value. Subsequent molecular dynamics studies indicate that in addition to the low mobility of surface-bound ions in the Stern layer, enhanced pairing and collisions between partially dehydrated ions of opposite charges also make important contributions to the reduced ion mobility. Furthermore, we show that the extent of mobility reduction depends on the association constant between cations and anions in different electrolytes with a more drastic reduction for a larger association constant." @default.
• W2912018790 created "2019-02-21" @default.
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• W2912018790 date "2019-02-16" @default.
• W2912018790 modified "2023-10-17" @default.
• W2912018790 title "Drastically Reduced Ion Mobility in a Nanopore Due to Enhanced Pairing and Collisions between Dehydrated Ions" @default.
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• W2912018790 doi "https://doi.org/10.1021/jacs.8b08488" @default.
• W2912018790 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6675019" @default.
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• W2912018790 hasPublicationYear "2019" @default.
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