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- W2912051347 endingPage "1044" @default.
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- W2912051347 abstract "Abstract A short asymmetric synthesis of an all‐ syn and all‐ trans kainoid core is reported. The synthetic route relies on the application of a new asymmetric [3+2] annulation reaction followed by a conjugate addition reaction to install this kainoid's three stereocenters. A surprising intramolecular conjugate addition enabled by the chiral tert ‐butylsulfinyl group residing on the 3‐pyrroline nitrogen atom surpassed its expected role as a steric spectator. Efforts to outcompete intramolecular 1,4‐addition by further oxidizing the sulfoxide, or use of additives, and advancement of the all‐ syn addition product to the requisite kainoid common core are detailed." @default.
- W2912051347 created "2019-02-21" @default.
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- W2912051347 date "2019-02-12" @default.
- W2912051347 modified "2023-10-12" @default.
- W2912051347 title "Efforts Toward a Unified Kainoid Family Synthesis Approach: Unexpected Sulfinamide‐Directed Conjugate Addition Results" @default.
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- W2912051347 doi "https://doi.org/10.1002/ajoc.201800728" @default.
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