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- W2912082435 abstract "Two new coordination assemblies were prepared by combining the open and close forms of 1,2-bis(5-carboxyl-2-methyl-3-thienyl)perfluorocyclopentene (H2dae) with [Mn2(saltmen)2(H2O)2](PF6)2, where H2saltmen = 2,2′-((1E,1′E)-((2,3-dimethylbutane-2,3-diyl)bis(azaneylylidene)) bis(methaneylylidene))diphenol. From X-ray diffraction analyses, the complexes had the following formula: [Mn2(saltmen)2(dae-open)] (1open) and [Mn(saltmen)(dae-close)]·H2O·Et3N (1close). Both complexes crystallized in the C2/c monoclinic space group. In 1open, dae-o2– behaves as a bidentate ligand attached to the outer Mn-saltmen monomer via the oxygen atom of carboxylato groups, whereas in 1close, the dae-c2– ligand behaves as a monodentate ligand attached to the external Mn-saltmen dimer by only one carboxylato group of the photochromic ligand. The complexes showed reversible photochromic responses to UV/vis light and showed single-molecule magnet-like behavior. The relaxation times and energy barriers of the metal complexes are clearly affected by UV/vis irradiation." @default.
- W2912082435 created "2019-02-21" @default.
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- W2912082435 date "2019-01-30" @default.
- W2912082435 modified "2023-10-06" @default.
- W2912082435 title "Synthesis, Structures, and Magnetic Properties of Two Coordination Assemblies of Mn(III) Single Molecule Magnets Bridged via Photochromic Diarylethene Ligands" @default.
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- W2912082435 doi "https://doi.org/10.1021/acs.inorgchem.8b02578" @default.
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