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- W2912105789 abstract "Abstract Catalysts of Ru and Ru−Au prepared by the wet impregnation and Deposition‐Precipitation methods supported on ZrO 2 modified by CeO 2 (10 and 20 wt%) synthetized by sol‐gel method, in order to study Au and CeO 2 addition effect in the catalytic wet air oxidation of phenol, carried out in an automatized continuous fixed‐bed reactor using oxygen as an oxidizing source. Characterizations of the catalysts were made by X‐ray Diffraction (XRD), Specific Surface Area (BET), X‐ray Photoelectron Spectroscopy (XPS), Transmission Electronic Microscopy ( TEM) , Scanning Electronic Microscopy (SEM), Ultraviolet – visible Spectroscopy (UV‐vis) and Temperature Programmed Desorption of Ammonia (NH 3 ‐TPD). The effect of Au is reflected in the selectivity to CO 2 of the catalysts Ru‐ZrO 2 and Ru−Au‐ZrO 2 with the increase in selectivity from 89 to 95% related to the increase in acidity which increases from 70 to 102 (μmol of NH 3 / gCat). Ce loading effect in this case was important to the enhance the CO 2 selectivity explained by the formation of Ce 4+ ‐O 2− ‐M that could favor the oxygen transfer between the catalyst surface and the adsorbed species by a redox mechanism." @default.
- W2912105789 created "2019-02-21" @default.
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- W2912105789 date "2019-01-25" @default.
- W2912105789 modified "2023-10-14" @default.
- W2912105789 title "Catalytic Wet Air Oxidation (CWAO) of Phenol in a Fixed Bed Reactor Using Supported Ru and Ru-Au Catalysts: Effect of Gold and Ce Loading" @default.
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- W2912105789 doi "https://doi.org/10.1002/slct.201802958" @default.
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