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- W2912120422 abstract "Nitrogen doping is a common approach for functionalization of graphene to generate active sites for catalytic reactions. However, the effect of nitrogen content and species within nitrogen-doped graphene (NG) on catalytic phenol oxidation remains largely unaddressed, especially for the peroxidisulfate (PDS) system. In this work, graphene (G), NH3•H2O-reduced graphene (NG-NH3), and N2H4-reduced graphene (NG-N2H4) with different nitrogen contents were synthesized, and their catalytic abilities in inducing PDS was evaluated. The degradation results indicated that nitrogen doping improved the catalytic ability of G and NG-NH3 shows a higher catalytic ability than NG-N2H4, even though they have similar nitrogen contents. Based on the XPS spectra, among all the doped nitrogen species, the graphitic N made the greatest contribution to the catalytic activity. The scavenger and electron paramagnetic resonance results imply a major contribution of a nonradical mechanism in the NG-PDS-phenol reaction system. Finally, the hydroquinone and p-hydroxybenzoic acid were identified as two intermediate products during the degradation. The decrease in total organic carbon concentration (TOC) after reaction confirmed that phenol was mineralized partially in CO2. These findings will guide the applications of NG as a catalyst and enrich our understanding of the PDS-phenol reaction system." @default.
- W2912120422 created "2019-02-21" @default.
- W2912120422 creator A5051336184 @default.
- W2912120422 creator A5058538136 @default.
- W2912120422 creator A5090741037 @default.
- W2912120422 date "2019-06-01" @default.
- W2912120422 modified "2023-10-18" @default.
- W2912120422 title "A nonradical reaction-dominated phenol degradation with peroxydisulfate catalyzed by nitrogen-doped graphene" @default.
- W2912120422 cites W1961453377 @default.
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- W2912120422 cites W1985269936 @default.
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- W2912120422 cites W2038245738 @default.
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- W2912120422 doi "https://doi.org/10.1016/j.scitotenv.2019.02.173" @default.
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- W2912120422 hasPublicationYear "2019" @default.
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