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• W2912122946 startingPage "21" @default.
• W2912122946 abstract "H2SO4 concentration has an important influence on the performance of vanadium electrolytes and flow batteries. However, the comprehensive research is still inadequate. In this work, a series of electrolytes with 1.5 M vanadium ions (V2+, V3+, V3.5+, VO2+ and VO2+) in various concentrations of H2SO4 (1.5 M, 2.0 M, 2.5 M, 3.0 M, 3.5 M and 4.0 M) are prepared and their physicochemical properties, electrochemical activities, single-cell performances, and static stability are studied in detail. The conductivity and viscosity of the electrolytes increase with increasing H2SO4 concentration. Besides, the electrochemical properties are improved in higher concentration of H2SO4 except for the charge transfer resistance and hydrogen evaluation reaction. Meanwhile, the single-cell performances with 3.0–4.0 M of H2SO4 are superior to those with 1.5–2.5 M of H2SO4. However, V3+ in 4.0 M H2SO4 is not stable enough to store for a long time at room temperature. The above results indicate that 3.0 M and 3.5 M of H2SO4 should be used as supporting electrolytes to achieve efficient and stable vanadium flow batteries. This work may also provide a guide for study and practical application of vanadium flow batteries." @default.
• W2912122946 created "2019-02-21" @default.
• W2912122946 creator A5032874982 @default.
• W2912122946 creator A5035900030 @default.
• W2912122946 creator A5043161993 @default.
• W2912122946 creator A5059197874 @default.
• W2912122946 date "2019-04-01" @default.
• W2912122946 modified "2023-10-11" @default.
• W2912122946 title "Revealing sulfuric acid concentration impact on comprehensive performance of vanadium electrolytes and flow batteries" @default.
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• W2912122946 doi "https://doi.org/10.1016/j.electacta.2019.02.062" @default.
• W2912122946 hasPublicationYear "2019" @default.
• W2912122946 type Work @default.
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