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• W2912140513 abstract "Abstract Direct valorization of methane to its alcohol derivative remains a great challenge. Photocatalysis arises as a promising green strategy which could exploit hydroxyl radical (·OH) to accomplish methane activation. However, both the excessive ·OH from direct H 2 O oxidation and the neglect of methane activation on the material would cause deep mineralization. Here we introduce Cu species into polymeric carbon nitride (PCN), accomplishing photocatalytic anaerobic methane conversion for the first time with an ethanol productivity of 106 μmol g cat −1 h −1 . Cu modified PCN could manage generation and in situ decomposition of H 2 O 2 to produce ·OH, of which Cu species are also active sites for methane adsorption and activation. These features avoid excess ·OH for overoxidation and facilitate methane conversion. Moreover, a hypothetic mechanism through a methane-methanol-ethanol pathway is proposed, emphasizing the synergy of Cu species and the adjacent C atom in PCN for obtaining C 2 product." @default.
• W2912140513 created "2019-02-21" @default.
• W2912140513 creator A5054295846 @default.
• W2912140513 creator A5073407872 @default.
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• W2912140513 date "2019-01-31" @default.
• W2912140513 modified "2023-10-16" @default.
• W2912140513 title "Direct functionalization of methane into ethanol over copper modified polymeric carbon nitride via photocatalysis" @default.
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• W2912140513 doi "https://doi.org/10.1038/s41467-019-08454-0" @default.
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