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• W2912145914 abstract "Abstract In this work a new method for inclusion of pressure effects in COSMO-type activity coefficient models is proposed. The extension consists in the direct combination of COSMO-SAC and lattice-fluid ideas by the inclusion of free volume in form of holes. The effort when computing pressure (given temperature, volume, and mole numbers) with the proposed model is similar to the cost for computing activity coefficients with any COSMO-type implementation. For given pressure, computational cost increases since an iterative method is needed. This concept was tested for representative substances and mixtures, ranging from light gases to molecules with up to 10 carbons. The proposed model was able to correlate experimental data of saturation pressure and saturated liquid volume of pure substances with deviations of 1.16% and 1.59%, respectively. In mixture vapor-liquid equilibria predictions, the resulting model was superior to Soave-Redlich-Kwong with Mathias-Copeman α-function and the classic van der Waals mixing rule in almost all cases tested and similar to PSRK method, from low pressures to over 100 bar. Good predictions of liquid-liquid equilibrium were also observed, performing similarly to UNIFAC-LLE, with improved responses at high temperatures and pressures." @default.
• W2912145914 created "2019-02-21" @default.
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• W2912145914 date "2019-06-01" @default.
• W2912145914 modified "2023-09-25" @default.
• W2912145914 title "A pairwise surface contact equation of state: COSMO-SAC-Phi" @default.
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• W2912145914 doi "https://doi.org/10.1016/j.fluid.2019.01.015" @default.
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