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- W2912151348 abstract "Two new layered complexes with the formulas of {[Cu(H 2 O)(HL) 2 Cl](NO 3 )} n ( 1 ) and {[Cu(H 2 O) 2 (HL) 2 ](NO 3 ) 2 } n ( 2 ) were solvothermally synthesized by the reactions of the bulky conjugated 4′‐(4‐hydroxyphenyl)‐4,2′:6′,4′′‐terpyridine ligand (HL) with different Cu II salts, which were further used as photocatalysts to achieve hydrogen production from water splitting. Single‐crystal structural analyses reveal that both complexes feature coplanar (4 4) layers with different connection manners between the HL extended Z‐shaped chains. More interestingly, 1 possessing more negative conduction band potential and higher structural stability exhibits a large hydrogen production rate of 2.43 mmol · g –1 · h –1 , which is four times higher than that of 2 . Thus, the Cu II ‐based coordination polymers modified by the bulky conjugated organic ligand can become potentially promising non‐Pt photocatalysts for hydrogen production from water splitting." @default.
- W2912151348 created "2019-02-21" @default.
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- W2912151348 date "2019-02-10" @default.
- W2912151348 modified "2023-10-12" @default.
- W2912151348 title "Two Bulky Conjugated 4′-(4-Hydroxyphenyl)-4,2′:6′,4′′-terpyridine-based Layered Complexes: Synthesis, Structure, and Photocatalytic Hydrogen Evolution Activity" @default.
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- W2912151348 doi "https://doi.org/10.1002/zaac.201800455" @default.
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