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- W2912158310 abstract "Abstract Nickel nanoparticles encapsulated in nitrogen-doped porous graphene (Ni@NPG) were synthesized through a one-pot method as a novel material for catalytic activation of persulfate (PS). The Ni@NPG catalysts were evaluated for adsorptive and catalytic removals of antibiotic sulfachloropyridazine (SCP) as an emerging pollutant and were found to exhibit excellent adsorption and catalysis with 100% SCP removal from water in only 30 min. Meanwhile, great stability and reusability can be achieved with satisfactory organic degradation after 4 successive runs. In addition, metal leaching was prohibited from the metal@carbon catalysts due to the protection of carbon walls. The influences of humid acid and inorganic anions (HCO3−, Cl−, Br− and H2PO4−) on SCP degradation at various concentrations were further investigated and the present study shows that all these species promoted the SCP degradation at a low concentration whereas an inhibition effect occurred at higher concentrations due to radical quenching. Electron paramagnetic resonance (EPR) and quenching experiments reveal the PS activation mechanism involving generation of SO4•−, •OH and •O2− without singlet oxygen. The synergistic effect of radical and nonradical pathways played crucial roles during the SCP oxidation process." @default.
- W2912158310 created "2019-02-21" @default.
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- W2912158310 date "2019-05-01" @default.
- W2912158310 modified "2023-10-17" @default.
- W2912158310 title "Nickel in hierarchically structured nitrogen-doped graphene for robust and promoted degradation of antibiotics" @default.
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- W2912158310 doi "https://doi.org/10.1016/j.jclepro.2019.01.323" @default.
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