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- W2912158728 endingPage "1762" @default.
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- W2912158728 abstract "Highly dispersed, core–shell Ni@Al2O3 on activated carbon (AC) catalysts were prepared to develop an effective, external-hydrogen-free fractionation process for various types of lignocellulosic biomass. In a mixture of formic acid, ethanol, and water at 190 °C, the conversion of oak wood produced 23.4 C% lignin-derived phenolic monomers (LDPMs) and highly delignified pulp-rich solid. At an early stage, formic acid acted as a cocatalyst to enhance the delignification by solvolysis, and at a later stage, it acted as a hydrogen source to stabilize the phenolic monomers by hydrodeoxygenation and hydrogenation. Based on the positive correlation between spillover hydrogen on the catalysts and LDPM yields, a new suite of catalyst design criteria was proposed to develop highly active, non-noble-metal based catalysts for realizing economically viable biorefineries. Enzymatic saccharification of the pulp-rich solid indicated that the pulp-rich solid is an excellent source of fermentable sugars." @default.
- W2912158728 created "2019-02-21" @default.
- W2912158728 creator A5010132153 @default.
- W2912158728 creator A5030593142 @default.
- W2912158728 creator A5038460242 @default.
- W2912158728 creator A5059575138 @default.
- W2912158728 creator A5071155383 @default.
- W2912158728 creator A5082315288 @default.
- W2912158728 date "2019-03-14" @default.
- W2912158728 modified "2023-10-14" @default.
- W2912158728 title "Fractionation of Lignocellulosic Biomass over Core-Shell Ni@Al<sub>2</sub> O<sub>3</sub> Catalysts with Formic Acid as a Cocatalyst and Hydrogen Source" @default.
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- W2912158728 doi "https://doi.org/10.1002/cssc.201802847" @default.
- W2912158728 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30702216" @default.
- W2912158728 hasPublicationYear "2019" @default.