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- W2912188752 abstract "The g-C3N4/SrTiO3 nanocomposite is an important material in photocatalysis, but little attention has been paid to their interfacial interaction in photocatalytic reaction. Herein, we prepare the g-C3N4/SrTiO3 nanocomposites via a two-step mechanically milling and calcination process. The composite exhibited the highest H2 evolution activity superior to that of the pure g-C3N4 and SrTiO3 in the visible light. The results of UV–vis DRS, PL and photoelectrochemical measurements demonstrated that g-C3N4/SrTiO3 exhibited more visible light adsorption and faster photo-generated charge transfer. Furthermore, the interfacial electronic structures of g-C3N4/SrTiO3 nanocomposites were thoroughly characterized. According to the XPS and DFT results, with the help of a strong built-in electric field presenting in the g-C3N4/SrTiO3 interface, the photo-generated electrons flow to the SrTiO3 from g-C3N4, leading to the highly-efficient electron separation and more H2O molecules photo-reduction to H2. This work explicates the significant role of built-in electric field in H2 evolution on g-C3N4/SrTiO3 photocatalyst." @default.
- W2912188752 created "2019-02-21" @default.
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- W2912188752 date "2019-06-01" @default.
- W2912188752 modified "2023-10-15" @default.
- W2912188752 title "Interfacial coupling effects in g-C3N4/SrTiO3 nanocomposites with enhanced H2 evolution under visible light irradiation" @default.
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- W2912188752 doi "https://doi.org/10.1016/j.apcatb.2019.01.089" @default.
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