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• W2912204532 endingPage "4035" @default.
• W2912204532 startingPage "4031" @default.
• W2912204532 abstract "A single device combining the functions of a CO2 electrolyzer and a formate fuel cell is a new option for carbon-neutral energy storage but entails rapid, reversible and stable interconversion between CO2 and formate over a single catalyst electrode. We report a new catalyst with such functionalities based on a Pb–Pd alloy system that reversibly restructures its phase, composition, and morphology and thus alters its catalytic properties under controlled electrochemical conditions. Under cathodic conditions, the catalyst is relatively Pb-rich and is active for CO2-to-formate conversion over a wide potential range; under anodic conditions, it becomes relatively Pd-rich and gains stable catalytic activity for formate-to-CO2 conversion. The bifunctional activity and superior durability of our Pb–Pd catalyst leads to the first proof-of-concept demonstration of an electrochemical cell that can switch between the CO2 electrolyzer/formate fuel cell modes and can stably operate for 12 days." @default.
• W2912204532 created "2019-02-21" @default.
• W2912204532 creator A5001451383 @default.
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• W2912204532 date "2019-02-14" @default.
• W2912204532 modified "2023-10-16" @default.
• W2912204532 title "An Integrated CO ₂ Electrolyzer and Formate Fuel Cell Enabled by a Reversibly Restructuring Pb–Pd Bimetallic Catalyst" @default.
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• W2912204532 doi "https://doi.org/10.1002/anie.201814257" @default.
• W2912204532 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30664835" @default.
• W2912204532 hasPublicationYear "2019" @default.
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