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- W2912227435 abstract "Abstract Design of novel non-precious polymers towards separation science is a fast-growing research point because of the need for high potential applications such as CO2 capture. Herein, we use four external cross-linkers (carbon tetrachloride, formaldehyde dimethyl acetal, α,α′-dichloro-p-xylene, 4,4′-bis(chloromethyl)-1,1′-biphenyl) to enhance the porosity of the polymeric adsorbents derived from the waste polystyrene. The best CO2 adsorption capacity and separation selectivity was achieved by the prepared adsorbents using carbon tetrachloride as the external cross-linkers (HCP-A). The CO2 adsorption capacity (2.521 mmol/g) at 1.0 bar and 273 K was achieved via the HCP-A adsorbents, which is 31.1% higher than the that of the adsorbents without using external cross-linkers (HCP-0). The BET surface area of HCP-A was 777 m2/g, which is 82.8% higher than that of HCP-0. In addition, the ideal separation selectivity (CO2/N2) was increased from 16.7 to 37.8 for the adsorbents after the introduction of the external cross-linkers." @default.
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- W2912227435 date "2019-04-01" @default.
- W2912227435 modified "2023-09-30" @default.
- W2912227435 title "Novel adsorbents derived from recycled waste polystyrene via cross-linking reaction for enhanced adsorption capacity and separation selectivity of CO2" @default.
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- W2912227435 doi "https://doi.org/10.1016/j.jtice.2019.01.014" @default.
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