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• W2912293336 abstract "The enols of 4-cyano-2,2,6,6-tetramethyl-3,5-heptanedione and of nitromalonamide were prepared as statistical mixtures of 18On (n = 0, 1, 2) isotopologues. The symmetries of their hydrogen bonds were probed by isotopic perturbation of their 13CO NMR signals. The former mixture shows a total of four signals, due to both intrinsic and perturbation isotope shifts. Therefore, that enol is a mixture of tautomers with an asymmetric hydrogen bond. In contrast, the mixture of isotopologues of nitromalonamide enol shows only two signals, due to an intrinsic isotope shift. Therefore, this is the first case, to be compared with the FHF– anion, of a neutral species with a single symmetric structure in solution and with a centered hydrogen." @default.
• W2912293336 created "2019-02-21" @default.
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• W2912293336 date "2019-02-08" @default.
• W2912293336 modified "2023-10-10" @default.
• W2912293336 title "Symmetry of Hydrogen Bonds in Two Enols in Solution" @default.
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• W2912293336 doi "https://doi.org/10.1021/jacs.8b13785" @default.
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