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- W2912308791 abstract "Significance Electron transfer (ET) is an elementary step in many chemical reactions and biological processes. Measuring ET at the single-molecule level opens new prospects for studying individual reaction steps and heterogeneity in ET. Despite recent advances, the connection between the single-molecule behavior and the ensemble averages remains unclear. By performing direct electrical measurements on ferrocene with variable lengths of molecular linkers, we found that the ET process is stochastic and follows first-order kinetics at the single-molecule level, but ensemble averaging of the single-molecule measurements recovers the thermodynamic behavior. This study provides a framework to connect stochastic single-molecule behavior and deterministic ensemble thermodynamics." @default.
- W2912308791 created "2019-02-21" @default.
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- W2912308791 date "2019-02-08" @default.
- W2912308791 modified "2023-10-12" @default.
- W2912308791 title "Transition from stochastic events to deterministic ensemble average in electron transfer reactions revealed by single-molecule conductance measurement" @default.
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- W2912308791 doi "https://doi.org/10.1073/pnas.1814825116" @default.
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