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- W2912331023 abstract "Highly efficient HPW(x)/MIL-100(Fe) catalysts with different phosphotungstic acid (HPW) loading (x, wt%) were successfully synthesized by a one-step hydrothermal method and characterized by XRD, SEM, FTIR, and BET. The influences of HPW loading, catalyst dosage, temperature, and O/S molar ratio on oxidative desulfurization (ODS) were investigated. The results indicated that the HPW(x)/MIL-100(Fe) retained the structure of its parent MIL-100(Fe). The MIL-100(Fe) presented a high surface area, which is beneficial to dispersion of HPW. The HPW(x)/MIL-100(Fe) with HPW loading of 40% exhibited excellent ODS activity. At a temperature of 50 °C, a catalyst dosage of 0.06 g, and an O/S molar ratio of 4, 100% desulfurization was achieved within 90 min for benzothiophene, dibenzothiophene, and 4,6-dimethyl-dibenzothiophene. The high catalytic activity of HPW(x)/MIL-100(Fe) can be attributed to highly dispersed HPW active sites with a high specific surface area." @default.
- W2912331023 created "2019-02-21" @default.
- W2912331023 creator A5020050167 @default.
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- W2912331023 date "2019-02-11" @default.
- W2912331023 modified "2023-10-14" @default.
- W2912331023 title "Synthesis of highly dispersed phosphotungstic acid encapsulated in MIL-100(Fe) catalyst and its performance in heterogeneous oxidative desulfurization" @default.
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- W2912331023 doi "https://doi.org/10.1080/00986445.2019.1573167" @default.
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