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• W2912352115 abstract "The nature of the glass transition is the self-organization of intermediate-range orders (IROs) in a supercooled liquid on cooling. This process was discussed on the basis of the three-step pathway for the nucleation and growth of crystalline solids such as IROs. The Suzuki scaling theory was applied to the nucleation process of a prenucleation cluster (PNC), the classical nucleation theory was applied to the nucleation process of primary particles and the classical crystal growth theory was applied to the growth process of a crystalline solid. The nucleation of PNCs in the first stage is a self-catalytic process, that is enhanced by boson peak modes in a supercooled liquid. The simulation of the crystal growth implies that the slow dynamics on cooling hinders a glass from becoming a crystal and permits IROs to coexist with an amorphous phase in a glass. The dissipative structure as the ultimate state of a glass is a thermodynamically stable state that is governed by the principle of Helmholtz free energy minimization as well as the equilibrium states of a liquid and crystal. This principle ensures the stable coexistence of IROs and an amorphous phase in a glass." @default.
• W2912352115 created "2019-02-21" @default.
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• W2912352115 date "2019-02-11" @default.
• W2912352115 modified "2023-09-27" @default.
• W2912352115 title "Slow dynamics on the self-organization of intermediate-range orders in a supercooled liquid and their stability in a glass" @default.
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• W2912352115 doi "https://doi.org/10.7567/1347-4065/aafb4c" @default.
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