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- W2912359915 abstract "The coordination-restricted ortho-site C-H bond activation and dehydrogenative homocoupling of 4,4'-(1,3-phenylene)dipyridine (1,3-BPyB) and 4,4'-(1,4-phenylene)dipyridine (1,4-BPyB) on different metal surfaces were studied by a combination of scanning tunneling microscopy, noncontact atomic force microscopy, and density functional theory calculations. The coupling products on Cu(111) exhibited certain configurations subject to the spatial restriction of robust two-fold Cu-N coordination bonds. Compared to the V-shaped 1,3-BPyB, the straight backbone of 1,4-BPyB helped to further reduce the variety of reactive products. By utilizing the three-fold coordination of Fe atoms with 1,4-BPyB molecules on Au(111), a large-scale network containing single products was constructed. Our results offer a promising protocol for controllable on-surface synthesis with the aid of robust coordination interactions." @default.
- W2912359915 created "2019-02-21" @default.
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- W2912359915 date "2019-02-11" @default.
- W2912359915 modified "2023-10-14" @default.
- W2912359915 title "Coordination-Controlled C–C Coupling Products via <i>ortho</i>-Site C–H Activation" @default.
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- W2912359915 doi "https://doi.org/10.1021/acsnano.8b06885" @default.
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- W2912359915 hasPublicationYear "2019" @default.
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