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- W2912376221 abstract "The combination of VCl3(THF)3 and N,N-bis(trimethylsilyl)aniline (1a) is an efficient catalyst for the [2+2+1] coupling reaction of alkynes and azobenzenes, giving multisubstituted pyrroles. A plausible reaction mechanism involves the generation of a mono(imido)vanadium(III) species as an initiation step, where 1a served as an imido source with concomitant release of 2 equiv of ClSiMe3, followed by a reaction with azobenzene to form a catalytically active bis(imido)vanadium(V) species via N═N bond cleavage." @default.
- W2912376221 created "2019-02-21" @default.
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- W2912376221 date "2019-02-07" @default.
- W2912376221 modified "2023-10-12" @default.
- W2912376221 title "Bis(imido)vanadium(V)-Catalyzed [2+2+1] Coupling of Alkynes and Azobenzenes Giving Multisubstituted Pyrroles" @default.
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- W2912376221 doi "https://doi.org/10.1021/jacs.8b13390" @default.
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