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• W2912400841 abstract "Cucurbit[7]uril (CB[7]) macrocycles exhibit a broad range of host-guest binding affinity. Attaching pendant CB[7] and complementary guests on 8-arm PEG macromers affords supramolecular hydrogels with cross-link affinity spanning more than 5 orders of magnitude (1.5 × 107 to 5.4 × 1012 M-1) without changing network topology. Cross-link affinity translates directly to bulk dynamic properties; hydrogels with high-affinity cross-linking behave like covalent gels with limited ability to relax or self-heal. Cross-link affinity furthermore dictates the release rate of encapsulated macromolecules, as well as cell infiltration and material clearance in vivo. This work thus informs a role for affinity in dictating supramolecular hydrogel properties by quantifying and isolating this feature over an unprecedented range." @default.
• W2912400841 created "2019-02-21" @default.
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• W2912400841 date "2019-02-01" @default.
• W2912400841 modified "2023-09-29" @default.
• W2912400841 title "Dynamic Supramolecular Hydrogels Spanning an Unprecedented Range of Host–Guest Affinity" @default.
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• W2912400841 doi "https://doi.org/10.1021/acsami.8b22151" @default.
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