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W2912404024 endingPage "2641" @default.
W2912404024 startingPage "2626" @default.
W2912404024 abstract "Simple, straightforward, and atom economic methods for the synthesis of quinolines, 2-aminoquinolines, and quinazolines via biomimetic dehydrogenative condensation/coupling reactions, catalyzed by well-defined inexpensive and easy to prepare singlet diradical Ni(II)-catalysts featuring two antiferromagnetically coupled singlet diradical diamine type ligands are described. Various polysubstituted quinolines, 2-aminoquinolines, and quinazolines were synthesized in moderate to good yields from different low-cost and readily accessible starting materials. Several control experiments were carried out to get insight into the reaction mechanism which shows that the nickel and the coordinated diamine ligands participate in a synergistic way during the dehydrogenation of alcohols." @default.
W2912404024 created "2019-02-21" @default.
W2912404024 creator A5002281773 @default.
W2912404024 creator A5019610146 @default.
W2912404024 creator A5038345349 @default.
W2912404024 creator A5063603305 @default.
W2912404024 creator A5070214324 @default.
W2912404024 creator A5071160860 @default.
W2912404024 creator A5087013376 @default.
W2912404024 date "2019-01-28" @default.
W2912404024 modified "2023-10-10" @default.
W2912404024 title "Dehydrogenative Synthesis of Quinolines, 2-Aminoquinolines, and Quinazolines Using Singlet Diradical Ni(II)-Catalysts" @default.
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W2912404024 doi "https://doi.org/10.1021/acs.joc.8b03070" @default.
W2912404024 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30685972" @default.