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- W2912453411 abstract "An efficient synthesis of highly functionalized cyclohexadienylborons via an inverse electron-demand Diels-Alder reaction/CO2 extrusion of alkenyl MIDA boronates with 2-pyrones is outlined. By controlling the reaction temperature, the corresponding C(sp3 )-rich bicyclolactones could also be readily formed. The exo-selective reactions feature good functional-group tolerance, broad substrate scope, and excellent regio- and diastereoselectivity. Oxidation of the cyclohexadienylborons in a one-pot procedure led to the construction of aromatic boronates bearing valuable functional groups. Synthetic transformations of the C-B bond were demonstrated." @default.
- W2912453411 created "2019-02-21" @default.
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- W2912453411 date "2019-02-22" @default.
- W2912453411 modified "2023-09-29" @default.
- W2912453411 title "Regio‐ and Diastereoselective Synthesis of Cyclohexadienylborons via an Intermolecular Diels–Alder Reaction of Alkenyl MIDA Boronates with 2‐Pyrones" @default.
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- W2912453411 doi "https://doi.org/10.1002/chem.201900011" @default.
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