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- W2912500113 abstract "Abstract Smythite ( ) is an iron‐based chalcogenide with a lamellar structure, different from the compositionally identical mineral greigite. Owing to their natural abundance, such transition metal chalcogenides are promising materials for low‐cost spintronic‐based devices. Herein, we discuss the charge transfer processes and complex magnetic ordering in a two‐dimensional (2D) smythite lattice. We find that redox couple and complex magnetic ordering are governing factors in the charge transfer processes. A very strong ferromagnetic in‐lattice coupling is also observed, which is attributed to the presence of three Fe‐centres. To describe the magnetic behaviour molecular and periodic approaches have been considered. We found a substantial increase in Curie temperature with applied mechanical stress due to opening of the double exchange interaction angle. We also observe an in‐plane Jahn−Teller distortion, which is further confirmed by the spin−orbit counter plot. Our study thus provides an insight into the double exchange mechanism favoured by the redox couple and results in a strong ferromagnetic ordering." @default.
- W2912500113 created "2019-02-21" @default.
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- W2912500113 date "2019-02-28" @default.
- W2912500113 modified "2023-09-23" @default.
- W2912500113 title "Double‐Exchange Magnetic Interactions in High‐Temperature Ferromagnetic Iron Chalcogenide Monolayers" @default.
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- W2912500113 doi "https://doi.org/10.1002/cphc.201900002" @default.
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