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• W2912511024 endingPage "1805737" @default.
• W2912511024 startingPage "1805737" @default.
• W2912511024 abstract "A “three birds, one stone” strategy is proposed to enhance the performance of hematite photoanode for photoelectrochemical water splitting. One-pot hybrid microwave synthesis of Ta and Sn codoped Fe2O3@FeTaO4 core–shell nanorods on F:SnO2 substrate achieves three synergetic effects simultaneously: i) core–shell heterojunction formation to alleviate the significant electron–hole recombination; ii) preserved morphology of small-diameter nanorods to provide a short hole diffusion distance; and iii) Ta and Sn codoping to enhance the electrical conductivity. These effects are not possible with conventional high temperature thermal synthesis in a furnace. As a result, core–shell Fe2O3@FeTaO4 electrode with FeOOH cocatalyst achieves a photocurrent density of 2.86 mA cm−2 at 1.23 VRHE under AM 1.5 G simulated sunlight (100 mW cm−2), which is ≈2.4 times higher than that of bare hematite (1.17 mA cm−2). In addition, the FeOOH/Fe2O3@FeTaO4 electrode exhibits a high surface charge separation efficiency of ≈85% and a modest bulk charge separation efficiency of ≈24%." @default.
• W2912511024 created "2019-02-21" @default.
• W2912511024 creator A5010021409 @default.
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• W2912511024 date "2019-01-28" @default.
• W2912511024 modified "2023-09-29" @default.
• W2912511024 title "Three Birds, One-Stone Strategy for Hybrid Microwave Synthesis of Ta and Sn Codoped Fe₂ O₃ @FeTaO₄ Nanorods for Photo-Electrochemical Water Oxidation" @default.
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• W2912511024 doi "https://doi.org/10.1002/adfm.201805737" @default.
• W2912511024 hasPublicationYear "2019" @default.
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