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• W2912541639 abstract "A Cu-azolate metal-organic framework (MOF) uptakes stoichiometric loadings of Groups 1 and 2 metal halides, demonstrating efficient reversible release and reincorporation of immobilized anions within the framework. Ion-pairing interactions lead to anion-dependent Li+ and Mg2+ transport in Cu4(ttpm)2·0.6CuCl2, whose high surface area affords a high density of uniformly distributed mobile metal cations and halide binding sites. The ability to systematically tune the ionic conductivity yields a solid electrolyte with a Mg2+ ion conductivity rivaling the best materials reported to date. This MOF is one of the first in a promising class of frameworks that introduces the opportunity to control the identity, geometry, and distribution of the cation hopping sites, offering a versatile template for application-directed design of solid electrolytes." @default.
• W2912541639 created "2019-02-21" @default.
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• W2912541639 date "2019-02-18" @default.
• W2912541639 modified "2023-10-16" @default.
• W2912541639 title "High Li⁺ and Mg²⁺ Conductivity in a Cu-Azolate Metal–Organic Framework" @default.
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• W2912541639 doi "https://doi.org/10.1021/jacs.8b13418" @default.
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