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• W2912557502 abstract "Adsorption of the carboxylic anchoring dye, p-ethyl red (p-ER), onto TiO2 nanoparticles in protic vs aprotic solvents was studied in situ using the surface-specific technique, second harmonic light scattering (SHS). Two different adsorption schemes were proposed to account for p-ER interactions with TiO2 under different solvent environments. In aprotic solvents, p-ER adsorbs directly onto TiO2. Conversely, in protic solvents, in which solvent molecules bind stronger than p-ER with TiO2, the dye molecules adsorb onto the solvent shell around the particle but not directly to the TiO2 surface. In addition, a portion of the p-ER molecules form hydrogen bonds with the protic solvent molecules. The two different adsorption models reproduce the measured adsorption isotherms detected by SHS. Specifically, the p-ER molecules adsorb with a smaller free energy change and a larger density in protic solvents than in aprotic solvents. Our results indicate that protic solvents are undesirable for administering adsorption of carboxylic dyes in dye-sensitized solar cell applications as the dye molecules do not directly adsorb onto the TiO2 particle." @default.
• W2912557502 created "2019-02-21" @default.
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• W2912557502 date "2019-02-06" @default.
• W2912557502 modified "2023-10-16" @default.
• W2912557502 title "Carboxylic Anchoring Dye <i>p</i>-Ethyl Red Does Not Adsorb Directly onto TiO₂ Particles in Protic Solvents" @default.
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• W2912557502 doi "https://doi.org/10.1021/acs.jpcc.8b08513" @default.
• W2912557502 hasPublicationYear "2019" @default.
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