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• W2912576088 abstract "Abstract Effective electrocatalysts are required for the CO 2 reduction reaction (CRR), while the factors that can impact their catalytic activity are yet to be discovered. In this article, graphitic carbon nitride (g‐C 3 N 4 ) is used to investigate the feasibility of regulating its CRR catalytic performance by interfacial electron transfer. A series of g‐C 3 N 4 /graphene with and without heteroatom doping (C 3 N 4 /XG, XG = BG, NG, OG, PG, G) is comprehensively evaluated for CRR through computational methods. Variable adsorption energetics and electronic structures are observed among different doping cases, demonstrating that a higher catalytic activity originates from more interfacial electron transfer. An activity trend is obtained to show the best catalytic performance of CRR to methane on C 3 N 4 /XG with an overpotential of 0.45 V (i.e., −0.28 V vs reverse hydrogen electrode [RHE]). Such a low overpotential has never been achieved on any previously reported metallic CRR electrocatalysts, therefore indicating the availability of C 3 N 4 /XG for CO 2 reduction and the applicability of electron transfer modulation to improve CRR catalytic performance." @default.
• W2912576088 created "2019-02-21" @default.
• W2912576088 creator A5028236459 @default.
• W2912576088 creator A5032628543 @default.
• W2912576088 creator A5034195419 @default.
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• W2912576088 date "2019-02-04" @default.
• W2912576088 modified "2023-10-15" @default.
• W2912576088 title "Impact of Interfacial Electron Transfer on Electrochemical CO ₂ Reduction on Graphitic Carbon Nitride/Doped Graphene" @default.
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• W2912576088 doi "https://doi.org/10.1002/smll.201804224" @default.
• W2912576088 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30714293" @default.
• W2912576088 hasPublicationYear "2019" @default.
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