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• W2912674222 endingPage "2170" @default.
• W2912674222 startingPage "2166" @default.
• W2912674222 abstract "Using solar energy to convert CO2 into valuable fuels or chemicals offers a powerful solution to urgent energy and environmental problems. However, the development of efficient and selective catalysts remains a considerable scientific challenge. To address this, catalytically active CoII centers can be anchored into the porous matrix of metal-organic frameworks (MOFs) by utilizing a robust Zr-based MOF (Zr-DMBD) functionalized with freestanding thiol groups to enable efficient post-synthetic metal insertion. The thus-prepared Zr-DMBD-Co MOF solids are modified by well-defined Co-thiolate units and have the capability of photocatalytically converting CO2 into CO with high efficiency and selectivity under visible-light irradiation in a water-containing system. The turnover number and CO selectivity reach as high as 97 941 and 98 %, respectively." @default.
• W2912674222 created "2019-02-21" @default.
• W2912674222 creator A5003661679 @default.
• W2912674222 creator A5039635290 @default.
• W2912674222 creator A5043307587 @default.
• W2912674222 creator A5054438192 @default.
• W2912674222 creator A5059038444 @default.
• W2912674222 creator A5062113076 @default.
• W2912674222 creator A5070735149 @default.
• W2912674222 date "2019-04-02" @default.
• W2912674222 modified "2023-09-26" @default.
• W2912674222 title "Anchoring Co ^II Ions into a Thiol‐Laced Metal–Organic Framework for Efficient Visible‐Light‐Driven Conversion of CO ₂ into CO" @default.
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