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• W2912676683 startingPage "185802" @default.
• W2912676683 abstract "In the present paper, we have carried out a comparative first principles as well as model Hamiltonian study to understand the novel magnetism in 6H perovskite iridates Ba3IrTi2O9 and Ba3TiIr2O9 resulting from an unusual combination of geometrical as well as exchange frustration owing to their unique crystal geometry. Our model calculations corroborated with multipolar analysis provides a comprehensive understanding of the spin-orbit entangled [Formula: see text] pseudo-spin states in both materials. While, the [Formula: see text] character is quite robust in the former compound, it is found to be directly related to the nature of magnetism in the latter iridate. The identification of the relevant spin model for the ideal structure of Ba3IrTi2O9 suggests that the Heisenberg exchange interaction dominates the Kitaev term favoring long range magnetic order in the system in line with the ab initio study while the other iridate Ba3TiIr2O9 has the posibility to host novel spin-orbital singlet state with no resultant moment." @default.
• W2912676683 created "2019-02-21" @default.
• W2912676683 creator A5005482229 @default.
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• W2912676683 date "2019-03-06" @default.
• W2912676683 modified "2023-09-24" @default.
• W2912676683 title "Spin–orbit coupling driven novel magnetism in d 5 6H-perovskite iridates Ba3IrTi2O9 and Ba3TiIr2O9" @default.
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• W2912676683 doi "https://doi.org/10.1088/1361-648x/ab048c" @default.
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• W2912676683 hasPublicationYear "2019" @default.
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