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• W2912702670 abstract "Rare earths, which are fundamental components of modern technologies, are often extracted from aqueous solutions using surfactants at oil-water interfaces. Heavier lanthanides are more easily extracted, even though all lanthanides are chemically very similar. Using x-ray fluorescence measurements and theoretical arguments, we show that there is a sharp bulk-concentration-dependent transition in the interfacial adsorption of cations from aqueous solutions containing Er^{3+} or Nd^{3+} in contact with a floating monolayer. The threshold bulk concentration of erbium (Z=68) is an order of magnitude lower than that of neodymium (Z=60), and erbium is preferentially adsorbed when the solution contains both ions. This implies that elemental selectivity during separation originates at the surfactant interface. Electrostatic effects arising from the interface dielectric mismatch, ionic correlations, and sizes of the ions explain the sharp adsorption curve and selectivity." @default.
• W2912702670 created "2019-02-21" @default.
• W2912702670 creator A5047781834 @default.
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• W2912702670 date "2019-02-08" @default.
• W2912702670 modified "2023-10-10" @default.
• W2912702670 title "Electrostatic Origin of Element Selectivity during Rare Earth Adsorption" @default.
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• W2912702670 doi "https://doi.org/10.1103/physrevlett.122.058001" @default.
• W2912702670 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30821995" @default.
• W2912702670 hasPublicationYear "2019" @default.
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