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- W2912705858 abstract "The delayed photofragmentation and photoelectron spectroscopy coupled with DFT calculations were employed for the investigation of the relaxation dynamics of m-xylene cations. The multiphoton ionization induced by the pump pulse was used for the preparation of the m-xylene cations, and the population was characterized by the technique of photoelectron imaging. A time-delayed probe pulse was used to excite the prepared m-xylene cations to energetically higher electronic states, which undergo fragmentation. The relaxation dynamics of the m-xylene cations was tracked by monitoring the depletion of excited parent-ion and the formation of the fragment-ion. Two relaxation time constants are determined by monitoring the depletion of the excited parent-ion and the formation of the fragment-ion with the delay time. The first component of τ1 = 764 (±25) fs is attributed to an intramolecular vibrational redistribution process within the D0 state and the slow one of τ2 > 440 ns is ascribed to the long lifetime of the cations." @default.
- W2912705858 created "2019-02-21" @default.
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- W2912705858 date "2019-02-12" @default.
- W2912705858 modified "2023-10-18" @default.
- W2912705858 title "Photoelectron imaging spectroscopy and photodynamics of m-xylene cations" @default.
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- W2912705858 doi "https://doi.org/10.1088/1612-202x/aaff52" @default.
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