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• W2912751587 abstract "The authors have developed low light-off temperature, hydrothermally stable catalysts for the removal of nitrogen oxide contaminants from lean-diesel emissions using hydrocarbon catalyzed selective catalytic reduction (SCR). This study utilizes the atomic layer deposition (ALD) technique to apply precisely controlled coatings onto metal ion exchanged zeolite particles to prepare drop-in ready catalysts with improved stability and activity. ALD was used to develop a bifunctional, core-shell coating on Cu-exchanged ZSM-5 particles, with ZrO2 deposited within the pore volume acting as a catalytic promoter in conjunction with an outer ZrO2/CeO2 layer for stabilization and to adsorb NOx. The core-shell ALD-catalyst synthesis approach demonstrated here provides a general strategy for a bifunctional zeolite stabilization and promotion. This work offers a pathway to minimize the usage of expensive rare earth metal oxides in the catalyst, providing an NOx removal strategy that mitigates emissions, storage, and corrosion concerns associated with ammonia SCR, the predominant SCR technology." @default.
• W2912751587 created "2019-02-21" @default.
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• W2912751587 date "2019-02-04" @default.
• W2912751587 modified "2023-10-18" @default.
• W2912751587 title "Hydrocarbon catalyzed-selective catalytic reduction catalysts using core-shell atomic layer deposited CeO₂ and ZrO₂" @default.
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• W2912751587 doi "https://doi.org/10.1116/1.5078646" @default.
• W2912751587 hasPublicationYear "2019" @default.
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