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• W2912802067 abstract "Layer-by-layer (LbL) assembly is widely applied as a coating technique for the nanoscale control of architecture and related properties. However, its translational applications are limited by the time-consuming and laborious nature of the process. Inspired by the blood-clotting process, herein, we develop a shear-flow-driven LbL (SF-LbL) self-assembly approach that accelerates the adsorption rate of macromolecules by mechanically configuring the polymer chain via a coil–stretch transition, which effectively simplifies and speeds the diffusion-controlled assembly process. The structural characteristics and surface homogeneity of the SF-LbL films are improved, and diverse three-dimensional structures can be achieved. Functional SF-LbL-assembled surfaces for corneal modification are successfully fabricated, and the surface of wounded rat corneas and skin can be directly decorated in situ with SF-LbL nanofilms due to the advantages of this approach. Furthermore, in situ SF-LbL self-assembly has promise as a simple approach for the wound dressing for interventional therapeutics in the clinic, as illustrated by the successful in situ fabrication of drug-free layers consisting of chitosan and heparin on the dorsal skin of diabetic mice to rescue defective wound healing. This bioinspired self-assembly approach is expected to provide a robust and versatile platform with which to explore the surface engineering of nanofilms in science, engineering, and medicine." @default.
• W2912802067 created "2019-02-21" @default.
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• W2912802067 date "2019-02-18" @default.
• W2912802067 modified "2023-10-15" @default.
• W2912802067 title "Bioinspired Shear-Flow-Driven Layer-by-Layer <i>in Situ</i> Self-Assembly" @default.
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• W2912802067 doi "https://doi.org/10.1021/acsnano.8b08151" @default.
• W2912802067 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30747513" @default.
• W2912802067 hasPublicationYear "2019" @default.
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