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- W2912814918 abstract "In the past two decades, the reaction mechanism of C-C bond formation from methanol or dimethyl ether (DME) has been intensively studied as the most critical problem of methanol to hydrocarbons (MTH) process, one of the most important reactions in C1 chemistry, but the first C-C bond generation during the very initial reaction stage remains a highly controversial issue. For the first time, a surface methyleneoxy-analogue, originated from the surface activated DME, was directly observed by in situ solid-state NMR and recognized to be the crucial intermediate for the first C-C bond formation in MTH process. In consequence, new insights into the first C-C bond formation were provided, suggesting DME/methanol activation and C-C bond direct formation via an interesting synergetic mechanism, involving C-H bond breakage and C-C bond coupling during the initial methanol reaction in the chemical environment of zeolite catalysis." @default.
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- W2912814918 date "2017-05-31" @default.
- W2912814918 modified "2023-10-15" @default.
- W2912814918 title "Direct Mechanism of the First Carbon-Carbon Bond Formation in the Methanol-to-Hydrocarbons Process" @default.
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- W2912814918 doi "https://doi.org/10.1002/ange.201703902" @default.
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