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- W2912860019 abstract "The focus of this thesis is the establishment and study of reversible electronic energy transfer (REET), following light excitation, between molecular subcomponents within ring-on-thread rotaxane nanometric architectures. When the lowest-lying chromophore excited states are quasi-isoenergetic and kinetics of interchromophore transfer are rapid, REET can be instilled - changing excited-state properties. Pyrene and ruthenium(II) tris(bipyridine) derivatives were chosen as matched chromophores. Rotaxane formation was based on active template copper catalysis (Huisgen and Cadiot-Chodkiewicz reactions) within a pyrene-decorated macrocycle, coupling half threads comprising bulky stopper groups - one of which being Ru(bpy)32+. Prolonged luminescence lifetimes (up to 14 μs), compared to parent Ru(bpy)32+, indicated that reversible electronic energy transfer processes were instilled in a series of rotaxanes of varying structure, which were studied by state-state and time-resolved spectroscopies." @default.
- W2912860019 created "2019-02-21" @default.
- W2912860019 creator A5027890810 @default.
- W2912860019 date "2018-09-05" @default.
- W2912860019 modified "2023-09-24" @default.
- W2912860019 title "Reversible electronic energy transfer in rotaxane architectures" @default.
- W2912860019 hasPublicationYear "2018" @default.
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