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• W2913008230 abstract "Despite its very high capacity (4200 mAh g-1), the widespread application of the silicon anode is still hampered by severe volume changes (up to 300%) during cycling, which results in electrical contact loss and thus dramatic capacity fading with poor cycle life. To address this challenge, 3D advanced Mxene/Si-based superstructures including MXene matrix, silicon, SiO x layer, and nitrogen-doped carbon (MXene/Si@SiO x@C) in a layer-by-layer manner were rationally designed and fabricated for boosting lithium-ion batteries (LIBs). The MXene/Si@SiO x@C anode takes the advantages of high Li+ ion capacity offered by Si, mechanical stability by the synergistic effect of SiO x, MXene, and N-doped carbon coating, and excellent structural stability by forming a strong Ti-N bond among the layers. Such an interesting superstructure boosts the lithium storage performance (390 mAh g-1 with 99.9% Coulombic efficiency and 76.4% capacity retention after 1000 cycles at 10 C) and effectively suppresses electrode swelling only to 12% with no noticeable fracture or pulverization after long-term cycling. Furthermore, a soft package full LIB with MXene/Si@SiO x@C anode and Li[Ni0.6Co0.2Mn0.2]O2 (NCM622) cathode was demonstrated, which delivers a stable capacity of 171 mAh g-1 at 0.2 C, a promising energy density of 485 Wh kg-1 based on positive active material, as well as good cycling stability for 200 cycles even after bending. The present MXene/Si@SiO x@C becomes among the best Si-based anode materials for LIBs." @default.
• W2913008230 created "2019-02-21" @default.
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• W2913008230 date "2019-02-05" @default.
• W2913008230 modified "2023-10-16" @default.
• W2913008230 title "MXene/Si@SiO_<i>x</i>@C Layer-by-Layer Superstructure with Autoadjustable Function for Superior Stable Lithium Storage" @default.
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• W2913008230 doi "https://doi.org/10.1021/acsnano.8b08821" @default.
• W2913008230 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30689350" @default.
• W2913008230 hasPublicationYear "2019" @default.
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