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- W2913206799 abstract "The electrochemistry of the Ni/NiCl2 electrode reaction was studied using Al/Na[AlCl4] -NaCl/NiCl2/Ni cell in which the capacities of the cell were limited by the Ni/NiCl2 electrode. The limiting mechanism of the electrode was found to be associated with the formation of NiCl2 on the surface of the nickel electrode. This phenomenon limits the mass transfer processes of the non-porous electrode and thus its area capacity density. Modifying the electrolyte with the NaBr and NaI additives was found to produce higher nickel utilization and lower impedance values due to doping effects, which is believed to open up the lattice for better mass transport. The solubility measurements indicate that the solubility of nickel chloride in the chloroaluminate melt is strongly dependent on the operational temperature of the cell and the chemical additives present in the electrolyte. The corrosion studies suggest that the nickel chloride material in the positive electrode is in thermodynamic equilibrium with the metallic constituent and, as a result, does not appear to attack current collector materials made of the same metal." @default.
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- W2913206799 date "2002-01-01" @default.
- W2913206799 modified "2023-10-14" @default.
- W2913206799 title "Fundamental Studies of Nickel Electrode in a Basic Na[AlCl4] Melt at 300°C" @default.
- W2913206799 doi "https://doi.org/10.1149/200219.0102pv" @default.
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