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• W2913307747 abstract "Abstract It is well known that upon electronic excitation various π-stacked dimers readily exhibit excimer formation, facilitated by a perfect sandwich-like arrangement between the chromophores. However, it is unclear whether such a dimer is also capable of electron transfer upon excitation, if a strong electron-donating group is covalently attached. In this work, we probe the nature of the excited state in a series of cofacially arrayed polyfluorene derivatives with electron-rich aromatic donor attached via a methylene linker. Our studies show that in all cases excimer formation is energetically favorable, and promotion of a charge-transfer state in such systems is possible but requires a free energy for electron transfer far exceeding 1 V. These findings shed light on important design principles for molecular scaffolds capable of stabilizing both excimeric and charge-transfer states upon their excitation." @default.
• W2913307747 created "2019-02-21" @default.
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• W2913307747 date "2019-04-01" @default.
• W2913307747 modified "2023-09-27" @default.
• W2913307747 title "Charge-transfer or excimeric state? Exploring the nature of the excited state in cofacially arrayed polyfluorene derivatives" @default.
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• W2913307747 doi "https://doi.org/10.1016/j.jphotochem.2019.01.030" @default.
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