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- W2913331866 abstract "Abstract Understanding the corrosion of nuclear waste glass is critical to predicting its safe disposal within a geological facility. The corrosion mechanisms and kinetics of the International Simple Glass, a simplified version of high-level nuclear waste glass, was shown to be significantly influenced by a high pH cement solution representative of disposal conditions. We provide the first microscopic characterisation of the porous, Zr-rich aluminoalkali-silica gel corrosion layer that was observed. Ca, Na and K from the cement solution were incorporated into the corrosion layer to charge compensate Si, Al and Zr species; the incorporation of Al was postulated to result in precipitation of an aluminosilicate-rich gel with large voids, facilitating rapid transport of species through the gel layer and significantly enhancing the corrosion rate. Precipitation of Al-containing zeolite and phyllosilicate phases was also observed, indicating that cementitious solutions may promote the detrimental ‘rate resumption’ stage of glass corrosion." @default.
- W2913331866 created "2019-02-21" @default.
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- W2913331866 date "2019-01-22" @default.
- W2913331866 modified "2023-10-01" @default.
- W2913331866 title "Influence of young cement water on the corrosion of the International Simple Glass" @default.
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- W2913331866 doi "https://doi.org/10.1038/s41529-018-0059-9" @default.
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